My favorites are the theme and mission summary. Tomb Raider: Legend has to have the best score of the series, in my opinion.
I prefer the original Tomb Raider score, the TR:Angel Of Darkness score and the TR: Anniversary score over Legend's score, still, it wasn't bad.
I have to agree with you. I realize now that the comment I made about TR: Legend having the best score was influenced by me thinking it was the funnest game of the series, however after playing it so often I found it was too linear. I only like the main theme and the mission summary from TR:L. I like the TRAOD score. It fit quite well with the overall feel of the game. Tomb Raider: Anniversary is my preferred score of the Tomb Raider series, with the original Tomb Raider score and TRAOD in second and Legend in third.
This is my favorite piece of score from Tomb Raider: Angel of Darkness from the first level, the
Parisian Ghetto. It gives the feel of mystery and invokes that kind of atmosphere ingame.